Spin-orbit Enabled Unconventional Stoner Magnetism

Sep 5, 2025
Intraband g-factors in UCoGe along the k line ( + k,  + k, 0:2) from DFT calculations. These g-factors quantify the energy splitting of Kramers doublets for fields applied along the x, y, and z directions. The value g = 1 corresponds to usual spin-1/2. Inset: Fermi surface of UCoGe. The g calculations are done along the arrow and for the bands producing the inner (pale red) Fermi surface.
Intraband g-factors in UCoGe along the k line ( + k, + k, 0:2) from DFT calculations. These g-factors quantify the energy splitting of Kramers doublets for fields applied along the x, y, and z directions. The value g = 1 corresponds to usual spin-1/2. Inset: Fermi surface of UCoGe. The g calculations are done along the arrow and for the bands producing the inner (pale red) Fermi surface.

The Stoner instability has long been recognized as a fundamental concept in the understanding of metallic ferromagnetic materials, capturing the interplay of Coulomb repulsion, Pauli exclusion, and twofold fermionic spin degeneracy. This paradigm was extended by demonstrating that the Stoner instability can be harnessed to generate unconventional magnetism, a class of magnetic materials characterized by momentum-dependent spin splitting.

These findings have far-reaching implications for the field of spintronics. This study finds that pseudospin can carry unexpected symmetries that precludes it from coupling to a Zeeman field. This phenomenon exists in materials with spin–orbit coupling and appears at the Brillouin zone boundary. With Coulomb repulsion, this spinless pseudospin phenomenon gives rise to Stoner instabilities into unconventional magnetism.

Authors

Michael Weinert and Daniel Agterberg (University of Wisconsin - Milwaukee)

Additional Materials

Designing Materials to Revolutionize and Engineer our Future (DMREF)